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The little thoughtful stuff was nice. Cordelia putting cinnamon in his blood was nice and thoughtful, if a little disgusting. Angel making her and Wesley breakfast. Angel letting her crash at his place when hers was infested. That was over and beyond because she was a terrible house guest.
Can't find a gif of it but the scene where the two of them are having coffee at the Bronze (I believe it's BTVS 1x07) is genuinely sweet and manage to singlehandedly make me like Angel 10x more. He just seems so happy and genuinely interested in what she has to say, and I love her ability to make him smile and laugh.